next up previous
Next: Acknowledgments Up: No Title Previous: Introduction

Experimental apparatus and high resolution measurements

The experimental apparatus, shown in detail in Fig. 1, is presently in use at the J.R. Macdonald laboratory. The spectrograph consists of a large hemispherical analyser with an inner radius tex2html_wrap_inline199  mm and outer radius tex2html_wrap_inline201  mm, a 40mm diameter 2-dimensional position sensitive detector (2D-PSD) made up of two MCP's, a resistive anode encoder (RAE) and a cylindrical 4-element lens mounted at the entrance of the analyser. The lens provides a virtual slit by focusing the incoming electrons down to a diameter of about 1 mm for improved energy resolution. The actual entrance slit (see Fig. 1) has a diameter of 6 mm to allow for the uninhibited passage of the primary ion beam. The lens is also used for decelerating the incoming electrons in the high resolution mode of operation. The hemispherical analyser has an overall acceptance energy range of 20 tex2html_wrap_inline203 and a mean energy resolution of 1 tex2html_wrap_inline203 (when the lens is focused under low resolution mode). Novel features include the use of an off-center entrance aperture placed at a non-zero entrance potential tex2html_wrap_inline207 . This has been found to improve the focusing properties of the spectrometer by compensating for fringing field effects, while enhancing the acceptance energy range[2].

   figure34
Figure: The Experimental Setup

Details of the spectrograph features, its operation to date, the electronics in use and the data acquisition system have been briefly reported in [2]. A full theoretical treatment of the electron trajectories in this non-typical hemispherical analyser will be reported elsewhere[4]. As we have not yet finished with the full characterisation of our spectrograph, we do not scan the voltages but keep them fixed on all elements including the lens. In particular, the lens voltages are determined to first order empirically in non-deceleration mode and then held fixed for all electrons with similar initial energies even when decelating. While this does not allow for the best results, it is a first step in exploring the many variable space of this 4-element lens.

Results are presented in Fig. 2 for two different ion charges which give rise to different projectile KLL Auger spectra. The data were corrected for dead time and were fitted with a Gaussian function superimposed on a theoretical curve based on the elastic scattering model (Binary Encounter electron (BEe) peak). The energy calibration was performed using an electron gun, while the beam energy was determined with high accuracy from the known energy of the F tex2html_wrap_inline209 (2p tex2html_wrap_inline211 line. The energy resolution is defined as tex2html_wrap_inline213 , where tex2html_wrap_inline215 is the initial energy, tex2html_wrap_inline217 the pass energy and tex2html_wrap_inline219 the deceleration factor. The spectra are very similar in quality with those already obtained for the same F tex2html_wrap_inline221 [5] and F tex2html_wrap_inline209 [6, 7] collision systems with a conventional tandem spectrometer. However, our new spectrometer is presently about a factor of 15-20 times more efficient even when having to run with ion beam currents of about 5nA imposed by deadtime limitations[3]. Typically, beam currents in zero-degree measurements using conventional tandem spectrometers can be about 20-100 times larger at 100-500nA depending on the collision system studied.

   figure48
Figure: High resolution projectile Auger spectra plotted as a function of the deceleration factor F: [Left] Double differential cross sections (DDCS) of the tex2html_wrap_inline197 Auger line produced by RTE in collisions of 21.75MeV F tex2html_wrap_inline229 H tex2html_wrap_inline231 , [Right] Normalized yield showing various KLL Auger lines produced in collisions of 21.78 MeV F tex2html_wrap_inline209 + He.

In Fig. 3 we plot the area under the F tex2html_wrap_inline209 (2p tex2html_wrap_inline183 ) line (single differential cross section or SDCS) as a function of the deceleration factor. This should remain constant under correct operation and constitutes one of the basic tests of any spectrometer. The area is seen to remain invariant (within the statistical error) for deceleration factors in the region of 2 up to 6 even in the present way of running the spectrograph and lens. The average value of the measured SDCS after transforming it to the projectile rest frame is tex2html_wrap_inline239  cm tex2html_wrap_inline183 /sr in good agreement with the best measurement to date using the KSU tandem spectrometer, having a value of tex2html_wrap_inline243   tex2html_wrap_inline245 , and with theory which predicts a value of tex2html_wrap_inline247   tex2html_wrap_inline245 [5].

In Fig. 3 it is seen that for large deceleration factors the resolution is not anymore proportional to 1/F (i.e. the pass energy). This is probably due to the fact that the lens voltages were kept constant at the value that determined the best focusing (or resolution) conditions for the case of no deceleration (F=1). At larger deceleration factors the size of the image at the entrance of the analyser (exit of the lens) as well as the angle of incidence of the electrons entering the analyser increases with increasing deceleration factor with a corresponding degradation of the energy resolution. Clearly we need to vary the voltages on the lens as the deceleration factor is changed. This will require the full characterization of the lens and will be done in the near future.

   figure66
Figure: Measurements of laboratory single differential cross sections (SDCS) of the tex2html_wrap_inline197 RTE line produced in collisions of 21.75 MeV F tex2html_wrap_inline221 + H tex2html_wrap_inline231 as a function of deceleration factor F: [Left] Variation of the area under the peak (SDCS) with F, [Right] Variation of relative energy resolution with F.

In conclusion we have shown that it is possible to use a single stage electron spectrometer with a position sensitive detector to perform high resolution measurements in the beam direction, thus minimizing kinematic broadening effects. This is made possible by using a large entrance aperture on a hemispherical analyser which allows for the uninhibited passage of the ion beam, thus avoiding large backgrounds from slit scattering. However, since a small entrance aperture is required for good resolution, a virtual slit was provided by focusing and decelerating electrons before entering the analyser by means of a 4-element lens. The feasibility of this idea is supported by the first test results presented here. Most important, our new apparatus has a much higher gain of about 15-20 over previously used tandem parallel-plate spectrometers and when equipped with a faster data detection/acquisition system a further gain of about 100 should be possible. In the future, when we have finished with the full characterization of our lens, we shall also be able to perform measurements of higher resolution, close to the limit of kinematic broadening.


next up previous
Next: Acknowledgments Up: No Title Previous: Introduction

Theo Tzouros
Wed Oct 14 12:01:08 EET 1998